Research Performance Progress Report [electronic resource]
The focus of this project was catalysis by ‘proton coupled electron transfer’ (PCET) to metal bound fragments derived from the most abundant small molecules (i. e. O<sub>2</sub> and N<sub>2</sub>). There are many important chemical challenges that are tied to this fundamental...
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| Online Access: |
Online Access |
|---|---|
| Format: | Government Document Electronic eBook |
| Language: | English |
| Published: |
Washington, D.C. : Oak Ridge, Tenn. :
United States. Department of Energy. Office of Basic Energy Sciences ; distributed by the Office of Scientific and Technical Information, U.S. Department of Energy,
2015.
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| Subjects: |
MARC
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| 245 | 0 | 0 | |a Research Performance Progress Report |h [electronic resource] |
| 260 | |a Washington, D.C. : |b United States. Department of Energy. Office of Basic Energy Sciences ; |a Oak Ridge, Tenn. : |b distributed by the Office of Scientific and Technical Information, U.S. Department of Energy, |c 2015. | ||
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| 500 | |a 11/30/2015. | ||
| 500 | |a "final project report #1" | ||
| 500 | |a Theopold, Klaus H. | ||
| 500 | |a Univ. of Delaware, Newark, DE (United States) | ||
| 513 | |a Final; | ||
| 520 | 3 | |a The focus of this project was catalysis by ‘proton coupled electron transfer’ (PCET) to metal bound fragments derived from the most abundant small molecules (i. e. O<sub>2</sub> and N<sub>2</sub>). There are many important chemical challenges that are tied to this fundamental reaction type. Among these are: metal catalyzed oxidations of organic molecules utilizing O<sub>2</sub> as the oxidant; reduction of O<sub>2</sub> to water close to the thermodynamic potential – in other words, the cathode of any fuel cell based on reactions with O <sub>2</sub>; transfer of reduced nitrogen species to organic substrates; fixation of nitrogen at modest temperatures and pressures. Any one of these problems has obvious implications for the generation and/or utilization of energy on a large scale. | |
| 520 | 0 | |a Catalysis; Small Molecule Activation; Pcet. | |
| 536 | |b FG02-92ER14273. | ||
| 650 | 7 | |a Inorganic, Organic, Physical, And Analytical Chemistry. |2 edbsc. | |
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| 710 | 1 | |a United States. |b Department of Energy. |b Office of Scientific and Technical Information. |4 dst. | |
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